Search results for "Conical nanopore"

showing 2 items of 2 documents

Biomolecular conjugation inside synthetic polymer nanopores via glycoprotein-lectin interactions

2011

We demonstrate the supramolecular bioconjugation of concanavalin A (Con A) protein with glycoenzyme horseradish peroxidase (HRP) inside single nanopores, fabricated in heavy ion tracked polymer membranes. Firstly, the HRP-enzyme was covalently immobilized on the inner wall of the pores using carbodiimide coupling chemistry. The immobilized HRP-enzyme molecules bear sugar (mannose) groups available for the binding of Con A protein. Secondly, the bioconjugation of Con A on the pore wall was achieved through its biospecific interactions with the mannose residues of the HRP enzyme. The immobilization of biomolecules inside the nanopore leads to the reduction of the available area for ionic tran…

NanometresSynthetic membraneTransport equationNanoporesInformation processingRectification propertiesCylinders (shapes)Materials TestingConcanavalin AGeneral Materials ScienceFunctional polymersConical nanoporeschemistry.chemical_classificationChemistryBlocking effectElectric rectifiersComputer simulationEnzymesData processingNanoporeEnzyme moleculesFunctional polymersMolecular imprintingPorosityBio-molecularInner wallsMolecular imprintingSupramolecular chemistryNanotechnologyHorseradish peroxidaseIonic transportsNanocapsulesBio-conjugationMoleculeParticle SizeAqueous solutionsGlycoproteinsBiomoleculesBioconjugationBiomoleculeNanostructuresModel simulationChemical engineeringModels ChemicalPolymer membraneConductance stateFISICA APLICADABiospecific interactionSynthetic polymersSugarsSupramolecular chemistryPore wallCarbodiimide-coupling chemistry
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Calcium binding and ionic conduction in single conical nanopores with polyacid chains: model and experiments.

2012

Calcium binding to fixed charge groups confined over nanoscale regions is relevant to ion equilibrium and transport in the ionic channels of the cell membranes and artificial nanopores. We present an experimental and theoretical description of the dissociation equilibrium and transport in a single conical nanopore functionalized with pH-sensitive carboxylic acid groups and phosphonic acid chains. Different phenomena are simultaneously present in this basic problem of physical and biophysical chemistry: (i) the divalent nature of the phosphonic acid groups fixed to the pore walls and the influence of the pH and calcium on the reversible dissociation equilibrium of these groups; (ii) the asym…

General Physics and AstronomyIonic bondingFunctionalizedDissociation (chemistry)Conical nanoporeNanoscale regionschemistry.chemical_compoundNanoporesI - V curveIonic conductivityGeneral Materials ScienceConical nanoporesPhosphonate groupCalcium concentrationChemistryGeneral EngineeringPH effectsPartition functionsIonic channelsIon equilibriumReversible dissociationChemical physicsFunctional groupsThermodynamicsDesalination membranesIon bindingPorosityDissociationBiophysical chemistryDissociation equilibriaInorganic chemistrychemistry.chemical_elementWater filtrationCalciumIonNernst-Planck equationsApplied potentialsIon bindingCarboxylationPhosphonic acidsComputer SimulationCarboxylateParticle SizeControlled drug releaseCurrent voltage curveIonsBinding SitesFixed charge densityPH sensitiveCarboxylic acidsDesalinationPhosphonic acid groupsPoly acidsElectric ConductivityCarboxylic acid groupsFixed ChargesNanostructuresCell membranesCurrent-voltage curvesModels ChemicalQuantum theoryFISICA APLICADACalciumBiological ion channelsCalcium bindingIonic currentCytologyPore wallStatistical mechanicsAcidsACS nano
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